Tunability of third order nonlinear absorption in (Pb,La) (Zr,Ti) O 3 thin films

D. Ambika; Viswanathan Kumar; C. S. Suchand Sandeep; Reji Philip

doi:10.1063/1.3534786

Tunability of third order nonlinear absorption in (Pb,La) (Zr,Ti) O ₃ thin films

D. Ambika^*
, Viswanathan Kumar
, C. S. Suchand Sandeep
, Reji Philip

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

12 Citations (Scopus)

Abstract

This paper reports the demonstration of the tunability of the third order nonlinear optical absorption in (Pb_1-3x/2 La_x) (Zr _0.53 Ti_0.47) (PLZT) thin films. The optical nonlinearity is investigated employing the open aperture z-scan technique at the off-resonant wavelength of 532 nm. By altering the defect chemistry in PZT through A-site aliovalent lanthanum substitution, the nonlinear optical (NLO) absorption can be effectively tuned. The results of the influence of lanthanum concentration on leakage current and microstructure have also been combined to confirm the defect-mediated mechanism of NLO absorption in PLZT thin films.

Original language	English
Article number	011903
Journal	Applied Physics Letters
Volume	98
Issue number	1
DOIs	https://doi.org/10.1063/1.3534786
Publication status	Published - 03-01-2011

All Science Journal Classification (ASJC) codes

Physics and Astronomy (miscellaneous)

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10.1063/1.3534786

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title = "Tunability of third order nonlinear absorption in (Pb,La) (Zr,Ti) O 3 thin films",

abstract = "This paper reports the demonstration of the tunability of the third order nonlinear optical absorption in (Pb1-3x/2 Lax) (Zr 0.53 Ti0.47) (PLZT) thin films. The optical nonlinearity is investigated employing the open aperture z-scan technique at the off-resonant wavelength of 532 nm. By altering the defect chemistry in PZT through A-site aliovalent lanthanum substitution, the nonlinear optical (NLO) absorption can be effectively tuned. The results of the influence of lanthanum concentration on leakage current and microstructure have also been combined to confirm the defect-mediated mechanism of NLO absorption in PLZT thin films.",

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AU - Ambika, D.

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AU - Suchand Sandeep, C. S.

AU - Philip, Reji

PY - 2011/1/3

Y1 - 2011/1/3

N2 - This paper reports the demonstration of the tunability of the third order nonlinear optical absorption in (Pb1-3x/2 Lax) (Zr 0.53 Ti0.47) (PLZT) thin films. The optical nonlinearity is investigated employing the open aperture z-scan technique at the off-resonant wavelength of 532 nm. By altering the defect chemistry in PZT through A-site aliovalent lanthanum substitution, the nonlinear optical (NLO) absorption can be effectively tuned. The results of the influence of lanthanum concentration on leakage current and microstructure have also been combined to confirm the defect-mediated mechanism of NLO absorption in PLZT thin films.

AB - This paper reports the demonstration of the tunability of the third order nonlinear optical absorption in (Pb1-3x/2 Lax) (Zr 0.53 Ti0.47) (PLZT) thin films. The optical nonlinearity is investigated employing the open aperture z-scan technique at the off-resonant wavelength of 532 nm. By altering the defect chemistry in PZT through A-site aliovalent lanthanum substitution, the nonlinear optical (NLO) absorption can be effectively tuned. The results of the influence of lanthanum concentration on leakage current and microstructure have also been combined to confirm the defect-mediated mechanism of NLO absorption in PLZT thin films.

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Tunability of third order nonlinear absorption in (Pb,La) (Zr,Ti) O ₃ thin films

Abstract

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