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Two-photon assisted excited state absorption in multiferroic YCrO 3 nanoparticles

  • Shiji Krishnan
  • , C. S. Suchand Sandeep
  • , Reji Philip
  • , Nandakumar Kalarikkal*
  • *Corresponding author for this work

    Research output: Contribution to journalArticlepeer-review

    Abstract

    We report a novel functionality for the ferroelectric-antiferromagnet YCrO 3 powder of optical limiting upon illumination by nanosecond laser pulses at 532 nm. The optical limiting properties are investigated using the open aperture z-scan technique. The obtained nonlinearity fits to a three-photon like absorption mechanism. It is proposed that this nonlinearity is caused by two-photon absorption, followed by excited state absorption. Two different sized samples were investigated and the nonlinearity is found to be size dependent.

    Original languageEnglish
    Pages (from-to)59-63
    Number of pages5
    JournalChemical Physics Letters
    Volume529
    DOIs
    Publication statusPublished - 09-03-2012

    All Science Journal Classification (ASJC) codes

    • General Physics and Astronomy
    • Physical and Theoretical Chemistry

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